No. Larousse does not offer legal free PDFs. However, they sometimes offer sample chapters (20-30 pages) via email newsletter sign-ups.
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Some users look for the 1st Spanish Edition from the 1970s, which may be out of print. While copyright still applies, some educators argue that abandonware (unavailable for purchase) justifies archival copies. However, legally, it is still infringement. it is still infringement.